Mechanisms of heavy metal immobilization and transformation during co-pyrolysis of pig manure with typical organic solid wastes.

Λεπτομέρειες βιβλιογραφικής εγγραφής
Τίτλος: Mechanisms of heavy metal immobilization and transformation during co-pyrolysis of pig manure with typical organic solid wastes.
Συγγραφείς: Zhao F; College of Energy, Xiamen University, Xiamen 361102, PR China; Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China; Guangdong Provincial Key Laboratory of High-Quality Recycling of End-of-Life New Energy Devices, Guangzhou 510640, PR China., Li D; Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China; Guangdong Provincial Key Laboratory of High-Quality Recycling of End-of-Life New Energy Devices, Guangzhou 510640, PR China., Chen H; Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China; Guangdong Provincial Key Laboratory of High-Quality Recycling of End-of-Life New Energy Devices, Guangzhou 510640, PR China., Zeng X; College of Energy, Xiamen University, Xiamen 361102, PR China. Electronic address: xianhai.zeng@xmu.edu.cn., Shan R; Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China; Guangdong Provincial Key Laboratory of High-Quality Recycling of End-of-Life New Energy Devices, Guangzhou 510640, PR China. Electronic address: shanrui@ms.giec.ac.cn., Lin L; College of Energy, Xiamen University, Xiamen 361102, PR China., Yuan H; Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China; Guangdong Provincial Key Laboratory of High-Quality Recycling of End-of-Life New Energy Devices, Guangzhou 510640, PR China., Chen Y; College of Energy, Xiamen University, Xiamen 361102, PR China; Guangzhou Institute of Energy Conversion, Chinese Academy of Sciences, Guangzhou 510640, PR China; Guangdong Provincial Key Laboratory of High-Quality Recycling of End-of-Life New Energy Devices, Guangzhou 510640, PR China.
Πηγή: Journal of hazardous materials [J Hazard Mater] 2026 Aug 01; Vol. 514, pp. 142739. Date of Electronic Publication: 2026 Jun 18.
Τύπος έκδοσης: Journal Article
Γλώσσα: English
Στοιχεία περιοδικού: Publisher: Elsevier Country of Publication: Netherlands NLM ID: 9422688 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1873-3336 (Electronic) Linking ISSN: 03043894 NLM ISO Abbreviation: J Hazard Mater Subsets: MEDLINE
Imprint Name(s): Original Publication: Amsterdam : Elsevier
Ιατρικοί όροι (MeSH): Manure*/analysis , Metals, Heavy*/chemistry , Solid Waste*, Charcoal/chemistry ; Refuse Disposal/methods ; Animals ; Pyrolysis ; Swine ; Spectroscopy, Fourier Transform Infrared
Περίληψη: The accumulation of heavy metals restricts the safe agricultural utilization of pig manure. Co-pyrolysis with organic additives offers a promising strategy to overcome the physicochemical defects of manure-derived biochar and enhance metal sequestration. This study investigated the co-pyrolysis of pig manure with distinct solid wastes including food residue, tea stems, and spent coffee grounds at 450-750 °C to elucidate heavy metal transformation mechanisms. Results demonstrated highly efficient immobilization for Cu, Cr, and Ni; specifically, in the tea stem co-pyrolysis biochar at 750 °C, the residual fractions of Cr and Ni reached 87.15% and 80.55%, respectively. Supported by X-ray diffraction (XRD) and Fourier transform infrared (FTIR) spectroscopy, this stabilization is driven by a dual pathway: direct precipitation into stable mineral phases such as Cu5FeS4 and MgCrO4, and surface complexation via persistent Si-O and C-O functional groups within the aromatized carbon network. Principal Component Analysis (PCA) confirmed that carbon skeleton aromatization and matrix alkalinity dictate the conversion of bioavailable fractions into inert residual forms. Conversely, Zn stabilization exhibited high temperature sensitivity, requiring over 650 °C for extensive mineralization. Furthermore, feedstock composition critically regulated metal fate: chloride-abundant food residue hindered Zn and Mn solidification by forming soluble chloro-complexes, whereas lignin-rich matrices significantly promoted biochar aromatization and porosity, reinforcing metal sequestration via enhanced cation-π interactions. Finally, comprehensive environmental risk evaluations revealed an asymmetrical characteristic of high total accumulation versus low ecotoxicity. Lignin-assisted high-temperature treatments effectively suppressed the ecological risk indices of the target metals, validating co-pyrolysis as a robust thermochemical strategy for the safe remediation and resource recovery of hazardous livestock waste.
(Copyright © 2026 Elsevier B.V. All rights reserved.)
Competing Interests: Declaration of Competing Interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper
Contributed Indexing: Keywords: Biochar; Co-pyrolysis; Heavy metal immobilization; Pig manure; Speciation; Transformation
Substance Nomenclature: 0 (Manure)
0 (Metals, Heavy)
0 (Solid Waste)
0 (biochar)
16291-96-6 (Charcoal)
Entry Date(s): Date Created: 20260619 Date Completed: 20260725 Latest Revision: 20260725
Update Code: 20260725
DOI: 10.1016/j.jhazmat.2026.142739
PMID: 42320099
Βάση Δεδομένων: MEDLINE
Περιγραφή
ISSN:1873-3336
DOI:10.1016/j.jhazmat.2026.142739