Academic Journal

Engineering dipole-dipole couplings for enhanced cooperative light-matter interactions

Λεπτομέρειες βιβλιογραφικής εγγραφής
Τίτλος: Engineering dipole-dipole couplings for enhanced cooperative light-matter interactions
Συγγραφείς: Burgess, Adam, Waller, Madeline C., Gauger, Erik M., Bennett, Robert
Στοιχεία εκδότη: American Physical Society
Έτος έκδοσης: 2025
Συλλογή: University of Glasgow: Enlighten - Publications
Περιγραφή: Cooperative optical effects are enabled and controlled by interactions between molecular dipoles, meaning that their mutual orientation is of paramount importance to, for example, superabsorbing light-harvesting antennas. Here we show how to move beyond the possibilities of simple geometric tailoring, demonstrating how a metallic sphere placed within a ring of parallel dipoles engineers an effective Hamiltonian that generates “guide-sliding” states within the ring system. This allows steady-state superabsorption in noisy room temperature environments, outperforming previous designs while being significantly simpler to implement. As exemplified by this showcase, our approach represents a powerful design paradigm for tailoring cooperative light-matter effects in molecular structures that extends beyond superabsorbing systems to a huge array of quantum energy transport systems.
Τύπος εγγράφου: article in journal/newspaper
Περιγραφή αρχείου: text
Γλώσσα: English
Relation: https://eprints.gla.ac.uk/357311/2/357311.pdf; Burgess, Adam, Waller, Madeline C. , Gauger, Erik M. and Bennett, Robert ORCID logoorcid:0000-0001-6931-8840 (2025) Engineering dipole-dipole couplings for enhanced cooperative light-matter interactions. Physical Review Letters , 134(11), 113602. (doi:10.1103/PhysRevLett.134.113602 ) (PMID:40192392)
DOI: 10.1103/PhysRevLett.134.113602
Διαθεσιμότητα: https://eprints.gla.ac.uk/357311/
https://eprints.gla.ac.uk/357311/2/357311.pdf
https://doi.org/10.1103/PhysRevLett.134.113602
Rights: cc_by_4
Αριθμός Καταχώρησης: edsbas.70C5E133
Βάση Δεδομένων: BASE